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The best of anime in no particular order, for the most part.

Best Soundtracks:

Kaiba(2008)
Cowboy Bebop(1999)
Ghost in the Shell(1995)
Akira(1988)
Legend of the Galactic Heroes(1997)
Ghost in the Shell: Stand Alone Complex(2003, 2005)
Laputa Castle in the Sky(1986)
Wolf's Rain(2003)
Haibane Renmei(2002)

Best animation:

Akira(1988)
Cowboy Bebop(1999)
Howl's Moving Castle(2004)
FLCL(2001)
Ghost in the Shell(1995)
Redline(2009)
Tengen Toppa Gurren Lagann(2007)
Ghost in the Shell: Stand Alone Complex 2nd GIG(2005)
Sword of the Stranger(2007)
Jin Roh: The Wolf Brigade (1998)

Best of the year:

2014: Gundam Unicorn, Parasyte, Kill la Kill
2013: Shinsekai Yori, Space Battleship Yamato 2199, The Wind Rises
2012: Fate/Zero(?), Hellsing Ultimate, Wolf Children
2011: Penguin Drum, King of Pigs(does it even count?), Black Lagoon: Roberta's Blood Trail
2010: Tatami Galaxy, Fullmetal Alchemist: Brotherhood, The Dissapearance of Haruhi Suzumiya
2009: Redline, Tokyo Magnitude 8.0
2008: Kaiba, House of Small Cubes, Detroit Metal City
2007: Death Note, Sword of the Stranger
2006: Ergo Proxy, Welcome to the NHK, The Girl Who Leapt Through Time, Diebuster
2005: Monster, GITS SAC 2nd GIG, Final Fantasy Advent Children
2004: Mind Game, Planetes, Re: Cutey Honey
2003: Princess Tutu, Tokyo Godfathers, Animatrix
2002: Haibane Renmei, The Cat Returns
2001: FLCL, Millenium Actress, GITS SAC

I haven't thought those lists through at all.