 If you liked
Chrno Crusade
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 ...then you might like
Elfen Lied
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Both are a deep dark horror/thriller animes with a unique blend of characters. Both certainly have their share of fan service and disturbing horror.
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Recommended by ShadowBlazer3000
They have a few themes in common, such as supernatural human-like creatures, action, romance, insane characters, and plenty of dramatic and tragic scenes, even though Elfen Lied is much more touching and disturbing.
Also, both anime involve horns and a sad brother-sister story.
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Recommended by RenaPsychoKiller