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If you liked Psycho-Pass add

...then you might like Mayoiga add

A much better mystery with crime and police elements instead of from a civilian prospective.

If you liked Soul Eater add

...then you might like Ao no Exorcist add

Both of the series follow an exorcist type story and both of the stories have a large scope. Both are also very action heavy but also very character and story driven.

If you liked Akira add

...then you might like Zankyou no Terror add

Both discuss politics, terrorism and the struggle of individuals in a broken society.

If you liked Hellsing add

...then you might like Afro Samurai: Resurrection add

Both are very action heavy and have very little story, and instead focus on their action

If you liked Hellsing add

...then you might like Afro Samurai add

Both are very violent and gory. Both also have little story and mainly focus on action. If you like Afro then you'll definitely like Hellsing.