 If you liked
Elfen Lied
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 ...then you might like
Kara no Kyoukai Movie 1: Fukan Fuukei
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Both are focused around a somewhat kawaii protagonist which both aquire the power to kill "anything" yet still manage to find worthy opponents
Both protagonists have some sort of emotional/mental flaws
Both protagonists "slice" limbs off their opponents
Both are supernatural and dark, full of gore with awesome music
Both protagonists have a male counter part
Both anime are focused around murder or deaths of lots of people
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Recommended by -FlameHaze-
Somewhat deep, interesting stories spiced up with blood and action. Similar themes
Both have a deep, calm, philosophical and amazing atmosphere, a lot of blood and violence but holding the incredibly competency to not be "too cruel to watch", letting a non-accostumed horror/violence anime' fan enjoy the show. Unfortunately, both also have predictable and poorly developed support characters.
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Recommended by ReinhardVonMusel
Similar for their eeriness, alternative approach to philosophical issues and use of violence
After elfen lied this was really the only anime that could somewhat compare. It has an incredibly good story, and should get that ending of Elfen Lied off your mind! ^^
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Recommended by Lucky_Dungeon
very similiar synopsis as in terms of character personalty Ryougi Shiki reminds me of Lucy a lot with her bloodlust an two personality's .The series has a very same haunting effect of music an ambient style,the music is quite beautiful actually in both series in Elfen lied when Lucy hums the main theme song you get this prickly feeling behind your neck it will stick you with for a while.If you like blood an gore an a twisted love story its an anime essential,just get used to heads twisting off an blood flowing everywhere an theres also Nudity.
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Recommended by ShinXShadow