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Here's some recommendations! Sorry, I'm not great at descriptions. (I'm @robot_problems on twitter btw)

https://myanimelist.net/anime/48/hack__Sign (The whole series is really good! One of the first people getting trapped in video game kinda thing.)
https://myanimelist.net/anime/1575/Code_Geass__Hangyaku_no_Lelouch (You probably already know, but might as well! World is taken over by one country and everyone is suppressed. One guy gets a power to get people to do what he wants so he kinda tries to help.)
https://myanimelist.net/anime/6746/Durarara (REALLY good! Gangs in Tokyo stuff. Every character's plot is somehow connect. Also has a bit of magic.)
https://myanimelist.net/anime/16592/Danganronpa__Kibou_no_Gakuen_to_Zetsubou_no_Koukousei_The_Animation (Killing game in a school kinda thing.)
https://myanimelist.net/anime/5630/Higashi_no_Eden (A game to make the world a better place but mc has no memories.)
https://myanimelist.net/anime/237/Koukyoushihen_Eureka_Seven (I'm in the middle of it now so I haven't quite got a handle on the plot but its mecha not sure aside from that)
https://myanimelist.net/anime/17247/Machine-Doll_wa_Kizutsukanai (Have dolls they control and fight at a school. Has some mystery to it too.)
https://myanimelist.net/anime/14513/Magi__The_Labyrinth_of_Magic (Have to defeat dungeons to get magic weapons. War between countries, etc.)
https://myanimelist.net/anime/21603/Mekakucity_Actors (A bunch of kids with eye powers (Drawing people's attention, telepathy, freezing people, etc.) Trying to figure out where they came from and making sure not to get killed. It's a bit confusing but really interesting if you stick with it.)
https://myanimelist.net/anime/14407/Persona_3_the_Movie_1__Spring_of_Birth (All of the Persona series is really good! These movies are the best though.)
https://myanimelist.net/anime/23755/Nanatsu_no_Taizai (Adventures with magic and trying to save the kingdom kind of stuff.)
https://myanimelist.net/anime/167/Scrapped_Princess (Prophecy told that princess will destroy the world. Everyone is trying to kill her, she's just trying to live. Turns into mecha stuff...)
https://myanimelist.net/anime/177/Tsubasa_Chronicle
https://myanimelist.net/anime/861/xxxHOLiC (I would recommend all of Tsubasa and xxxHolic but it might be a little confusing without watching at least some of Cardcaptor Sakura first. I would give it a try without watching it though if you want to! This is all Clamp universe which gets a bit complex.)

I hope this helps and you find something you like! I'd also be happy to answer any questions about them.