 If you liked
Trigun
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 ...then you might like
No.6
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Both are Science Fiction anime mixing futuristic tech as well as showing desert-like wasteland environments, and focus on the moral dissonance between optimism and cynicism, angels and devils, pacifism and practicality. In this respect Nezumi/Rat and Wolfwood both act as the cynical ones, who have disdain for Shion and Vash's optimism and pacifism, but are ultimately converted. They have very different stories, but both portray a lot of the same themes of peace and compassion for human life, the value of relationships between people, and humanity's capacity for both great good and great evil.
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Recommended by noirgrimoir