 If you liked
Elfen Lied
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 ...then you might like
Darker than Black: Kuro no Keiyakusha
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They're both dark Animes... they have really lovable villains... and in DTB the main character kinda has split personalities too... Elfen Lied's the bloodier of the two.. but if you like one of them... the other is worth checking out ^^
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Recommended by StabbyPWNS
Hei and Lucy are similar in their personalities. Hei is very violent with his mask on similar to how lucy is. but when hei takes his mask off he becomes one of most gentle people alive with the given name lee like how nyuu is. They both use different names when their other split personality takes over. nevertheless, hei and lucy were both controlled by agency and rebelled against them and tried to eliminate them.
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Recommended by lexdemon514