 If you liked
Majin Tantei Nougami Neuro
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 ...then you might like
Ansatsu Kyoushitsu
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-Lets strat with the most obvious in those both seires, they are both have the same mangaka Yuusei, Matsui.
-Both shows the seek to know the ULTIMATE Mystorious thing in the storyline such as "who really is koro-sensei?" or on ther other show - "what really happned to Yako's father?" and so on...!
-Both animes has a "Unique" main character which isn't like any other regular person
-Both main character can't be actually identifed as Good or Bad personallity as for their S (Sadistic) side of them, or on the other side, to destroy Earth (ansatsu kyoushitsu).
-Both seires has a villain with an unknown personallity or past or
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