 If you liked
Seisenshi Dunbine
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 ...then you might like
Gundam: G no Reconguista
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Both have similar plots where the main character starts off as a member of a one faction, but quickly defects to a freedom fighter/rebel group-type faction where he stays for the rest of the show. Both shows are also directed by Yoshiyuki Tomino, and share many of the quirks of his style. Dunbine is a much easier watch, as it is paced more evenly, while G-Reco is paced very quickly and requires the viewer's full attention.
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Recommended by FinalReality56