Suzumiya Haruhi no Yuuutsu, Maria†Holic Recommendations
Haruhi and mariya... both bullies, the walk, the look, the wink... all the same
Matsurika and nagato... both w/ the emotionless personality
Mikuru and Kanako... the ones being bullied
Different Plots, but they have similar character characteristics....
The relations between the characters are quite similar: in both anime we have the bully (Haruhi/Mariya), the one being bullied (Mikuru/Kanako), and the silver-haired smart kuudere who just doesn't care (Yuki/Matsurika).
Also, both series are set at school and have comedy and parody.