Total Recommendations: 1
If you liked
Kidou Tenshi Angelic Layer
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...then you might like
Chobits
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The plots of both these anime originate from the same manga-ka, and deal with the relationships that can develope between humans and machines. They are both very sweet and very emotional with a little bit of humour thrown in. Chobits is a bit more mature, however, and has a darker tone to the plot at times.