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If you even have one, sometimes the OST's are just that good to listen to. I personally prefer
Such a lovely song. Sets the mood perfectly so much that I was almost brought to tears just by hearing it...but you'll have to do better than that to make me cry.

Edit: If it reminds you of something (besides the anime LOL) be sure to tell us.

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Soundtrack would be 'Keep the Beats!' from Angel beats! Does that count?

I have so many i don't even know where to begin.

Let's begin with Aria

I get the OSts for any good anime I watch here are my top 15:

1."What's Justice?" - Code Geass R2 OST2
2. Chokkaku - Bleach Movie 4 OST
3. Kouken - Naruto Shippuden OST2
4. Banjiya Blues - Gintama OST2
5. Stories - Code Geass OST
6. Theme of SSS - Angeal Beats OST2
7. Nothing Can be Explained - Bleach OST
8. Fairy Tail Main theme (Metal) - Fairy Tail OST2
9. Virals theme - Gurren Lagann OST
10. Vegetas Theme - DBZ OST
11. Awaken - Samurai Deeper KYO OST
12. Power up - HSD Kenichi OST
13. Orochimarus Theme - Naruto OST
14. Sadness and Sorrow - Naruto OST
15. Black Stars theme - Soul Eater OST

Thats all I have on my iPod at the moment, all of these are high class OSTs.

Off the top of my head...

-Madoka Magica OST
-5 cm per Second OST
-Panty and Stocking OST
-Zoku Natsume Yuujinchou OST
-Angel Beats! OST
-Karigurashi no Arrietty OST
-Clannad OST

All of these are lovely soundtracks, many of them containing some of my most loved tracks.

Too many to list. Off the top of my head:

Noir - Canta per me, Salva nos
Saraiya Goyou - Umaku Ikusa, Hisoyaka Ni.
Shiki - almost the entire OST. Eau de vie and Epitaph, most notably.
Evangelion - Thanatos, Komm Süsser Tod.
Ghost in the shell (SAC) - Torukia, Making of a Cyborg
Beck - Moon on the water
Aria - Barcarolle
Kara no Kyoukai - M12+13, M23
Read or Die - The main theme of R.O.D
Cossette no Shouzou - Somewhere I belong

Right now a few tracks from the Ao no exorcist OST.

I have too many to name myself, so I'll just list a top ten in no particular order featuring my favorite songs from each...

Bubblegum Crisis-Konya Wa Hurricane
Dirty Pair Flash-Kokoro De Mitsumeteru
Gall Force-Good Feeling
Gunbuster-Active Heart
Iczer-One-Eien no Iczer-One
Kanon 2006-Last Regrets
Macross-Tenshi no Enogeru
Megazone 23-Senaka Goshi Ni Sentimental
Neon Genesis Evangelion-Cruel Angels Thesis
Sakura Taisen-Yume Mite Iyou

Several tracks from OST's of Azumanga Daioh, Berserk, Death Note, Fate/Stay Night, Higurashi no Naku Koro ni, Mushishi, Noir and Shiki.

Out of all, the best OST is Noir's, hands down.

Tsuka no Ma no Shiawase from Katekyo Hitman Reborn... so relaxing...

I like many OST in anime but the only ones that i've loved enough to actually have made me buy/download them are:

1. Cowboy Bebop OST (yep all 9 discs)
2. Angel Beats! OST (Jun Maeda did a great work also...GirlDeaMo RULEZ!)
3. Nodame Cantabile OST (Put me in touch with that classic side i've forgotten for some time)
4. Naruto OST (some kickass fighting music i recall)
5. Samurai Champloo (Sick hip-hop beats...thx Nujabes RIP)

Madoka OST is really cool, for example:

This
Or this.

And Magia

*fap* *fap* *fap*

I have a lot but I'll just name 2

Chicken Bone: Cowboy Bebop

1. Madoka magika
2. Fairy tail.
3. Emma, a Victorian Romance
4. Tsubasa chronicle

Mobile Suit Gundam 00
Seirei no Moribito
Fate/stay night: Unlimited Blade Works

Basically anything composed by Kawai Kenji.

I like...
1.) Inu-Yasha
http://youtu.be/qijpOmkrGAI

2.) Arjuna
http://youtu.be/LJV6jAyfOs4

3.) .Hack//Sign
http://youtu.be/EfwJOyfmXj4

(Zoku) Natsume Yuujinchou entire OST. But this one stands out
http://www.youtube.com/watch?v=sCSKZnpTNNE
Last Exile entire OST

Mushishi entire OST

Eh, I have way too many actually.

Right now I haven't really been listening to soundtracks to anime but I have always loved The Girl Who Leapt Through Time OST.

Mine are:

Soundscape to ardor (bleach)
Beware of guys who use Umbrellas on sunny days (gintama)
Haru to Usobuko (mushishi)
The Last Wolf Suite (Rurouni Kenshin)

As much as I find the anime overrated I absolutely love the OST of Death Note. I've listened to it quite a bit.